El Hazard (All 4 Series)
Tenchi Muyo (All Series/Spinoff 10)
Ah! My Goddess
Aquarion OVA (forget the Anime...didn't make much sense. OVA was Better)
Cowboy Bebop
Dual Parallel Adventure
Flame of Recca (Manga Recommended)
Full Metal Panic (Start reading FMP Sigma after The Second Raid)
Gate Keepers
Gate Keepers 21
Gun X Sword
Guyver - The Bioboosted Armour
Hack Roots
Now and Then, Here and There (really dark stuff)
Rurouni Kenshin
The Law of Ueki
Trigun
Tsubasa Chronicle (Manga Recommended)
Vandread
XXXHolic (Manga Recommended)
.hack Quantum
Air Gear OVA (Anime was OK but...manga recommended)
Akikan (skip it, read the novel)
Angel Beats
Ano Hana
Ano Natsu
Another
Ao no Exorcist
Armored Trooper VOTOMS (watching series not required)
Baccano!
Baka to Test (Series and OVA)
Bakemonogatari
BALDR Forve EXE
Ben-to
Birdy the Mighty Decode
Black Blood Brothers
Black Rock Shooter
Boku Ha Tomodachi
Break Blade
Bus Gamer
Busou Shinki Moon Angel
Card Captor Sakura
Carnival Phantasm
Cat Shit One (OMG must watch)
Clannad (Will make you f*cking cry)
Code Geass (#1 in top 3)
D. Gray Man (Read Manga after anime ends)
Darker than Black (#2 in Favorite anime after that read the manga
Prequel http://vatoto.com/comic/_/comics/darker-than-black-kuro-no-keiyakusha-r1411
After Season 1 http://vatoto.com/comic/_/comics/darker-than-black-shikkoku-no-hana-r1414
Then Watch Darker Than Black Gaiden and after that Darker Than Black Gemini of the Meteor!!!!!!)
Deadman Wonderland (Manga Recommended)
Devil May Cry (Passable)
Dogs Bullet and Carnage (meh)
Durarara!!
Eden of the East (Priority)
EF A Tale of Memories
EF A Tale of Melodies
Eureka Seven
Fate Series
FLCL
FMA - Brotherhood
Ga-REi Zero
Ghost in the Shell
Guilty Crown
Gundam 00
Gundam MS IGLOO
Gundam Unicorn
Hatsukoi Limited
Hayate no Gotoku
Highschool of the Dead
Isekai no Seikishi Monogatari (#4 Favorite)
Katanagatari (#5)
Kenichi (Manga after series finish)
Kimi ni Todoke (Manga after Anime)
Kobato (Will make you cry)
Kore wa Zombie desu ka?
Kuragehime (a sleeper hit, read manga after anime finished)
Kurokami
Kuroshitsuji (some shounen ai but tolerable)
Level E
Mawaru Penguindrum
Megane no Kanojo
Mirai Nikki
Nagasarete (manga after anime)
Natsume Yuujinchou (#6 Favorite...so heart aching)
Nichijou
Nisemonogatari
Nyan Koi
Phantom Requiem for the Phantom
School Days (So much Drama)
Scrapped Princess
Sekirei (Manga after anime season 1)
Shakugan no Shana (I II then S then III)
Sora no Otoshimono
Soul Eater (Manga after episode 30+)
Spice and Wolf
Straight Jacket
Haruhi Suzumiya
Tales of Phantasia
Tales of Symphonia
The Sacred Blacksmith (read the novel/manga)
The World God Only Knows
Thundercats
Tiger and Bunny
To Aru Kagaku no Railgun (Manga waaay better)
To Aru Majutsu no Index (#3!!!! Favorite)
Towa no Quon
Usagi Drop (Manga much better coz Anime stopped halfway. Animation is good though)
Working!!
Xam'd Lost Memories
Movies
Cowboy Bebop Knockin' on Heaven's Door
xxxHOLIC - A Midsummer Nights Dream
Trigun - Badlands Rumble
Ah My Goddess
FF VII Advent Children
Highlander - The Search for Vengeance
Tsubasa Chornicle
Rurouni Kenshin
Resident Evil Degeneration
5 cm/sec (Favorite Movie of all time)
Akira
Appleseed
Appleseed Ex Machina
Beyond the Clouds, The promised place
Bungaku Shoujo (be sure to watch OVA first)
Children Who Chase Lost Voices from Deep Below
Daft Punk - Interstella 5555 - the 5tory of the 5ecret 5tar 5ystem
Deathnote Live Action
Detroit Metal City Live Action
Eden of the East (after anime)
Fate Stay Night
FMA - The Sacred Star
Gundam 00 - Awakening (after anime)
Halo Legends
Hayate - Heaven is a place on earth
Hotarubi no Mori e
Kara no Kyoukai
Karas (highly recommended)
Mardock Scramble
Neon Genesis Evangelion (Don't watch anime...will piss you off)
Origin Spirits of the Past
Pale Cocoon
Princess Mononoke
Robotech - Shadow Chronicles
Sora no Otoshimono
Summer Wars
Sword of the Stranger
Tales of Vesperia - First Strike
Tekken Blook Vengeance
The Borrower Arrietty
Disappearance of Suzumiya Haruhi
The Girl who Leapt Through Time
The Princess and the Pilot
Time of Eve
Vexille
Voices of a Distant Star
Please don't include new anime coz I'm still watching it and haven't placed it in the list yet